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Chemical vapour deposition of 1H,1H,2H,2H-Perfluorooctyltriethoxysilane (PFOES) to the unmodified TEMPO-oxidized aerogels was performed to remodel the amphiphilic cellulose to the a single with the hydrophobic surface area by way of silane functionalization from the cellulose nanofibres. The unmodified TEMPO-oxidized cellulose nanofibre aerogel was